Issue 64, 2015
From the journal:

Chemical Communications

Real time chemical imaging of a working catalytic membrane reactor during oxidative coupling of methane†

A. Vamvakeros,ab   S. D. M. Jacques,*bc   V. Middelkoop,*d   M. Di Michiel,e   C. K. Egan,c   I. Z. Ismagilov,f   G. B. M. Vaughan,e   F. Gallucci,g   M. van Sint Annaland,g   P. R. Shearing,h   R. J. Cernikc  and  A. M. Beale*ab  

* Corresponding authors

a Department of Chemistry, University College London, 20 Gordon Street, London WC1H 0AJ, UK
E-mail: andrew.beale@ucl.ac.uk

b UK Catalysis Hub, Research Complex at Harwell, Harwell, Didcot, Oxon, UK

c School of Materials, University of Manchester, Manchester, Lancashire M13 9PL, UK
E-mail: simon.jacques@gmail.com

d Flemish Institute for Technological Research, VITO NV, Boeretang 200, Mol, Belgium
E-mail: vesna.middelkoop@vito.be

e ESRF, 6 Rue Jules Horowitz, 38000 Grenoble, France

f Boreskov Institute of Catalysis SB RAS, Pr. Akademika Lavrentieva 5, 630090 Novosibirsk, Russia

g Chemical Process Intensification, Department of Chemical Engineering, Eindhoven University of Technology, Box 315, Eindhoven, Netherlands

h Department of Chemical Engineering, University College London, Torrington Place, London WC1E 7JE, UK

Abstract

We report the results from an operando XRD-CT study of a working catalytic membrane reactor for the oxidative coupling of methane. These results reveal the importance of the evolving solid state chemistry during catalytic reaction, particularly the chemical interaction between the catalyst and the oxygen transport membrane.

Graphical abstract: Real time chemical imaging of a working catalytic membrane reactor during oxidative coupling of methane

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Article information

DOI
https://doi.org/10.1039/C5CC03208C
Article type
Communication
Submitted
17 Apr 2015
Accepted
27 May 2015
First published
28 May 2015
This article is Open Access
Creative Commons BY license

Chem. Commun., 2015,51, 12752-12755

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Real time chemical imaging of a working catalytic membrane reactor during oxidative coupling of methane

A. Vamvakeros, S. D. M. Jacques, V. Middelkoop, M. Di Michiel, C. K. Egan, I. Z. Ismagilov, G. B. M. Vaughan, F. Gallucci, M. van Sint Annaland, P. R. Shearing, R. J. Cernik and A. M. Beale, Chem. Commun., 2015, 51, 12752 DOI: 10.1039/C5CC03208C

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