Experimental and theoretical investigation of a stable zinc-based metal–organic framework for CO2 removal from syngas

Ruiqin Zhong; Jia Liu; Xing Huang; Xiaofeng Yu; Changyu Sun; Guangjin Chen; Ruqiang Zou

doi:10.1039/C5CE01320H

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Experimental and theoretical investigation of a stable zinc-based metal–organic framework for CO₂ removal from syngas†

Ruiqin Zhong,*^a Jia Liu,^b Xing Huang,^a Xiaofeng Yu,^a Changyu Sun,^a Guangjin Chen^a and Ruqiang Zou*^b

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* Corresponding authors

^a State Key Laboratory of Heavy Oil Processing, China University of Petroleum, Beijing 102249, China
E-mail: rzhong@cup.edu.cn

^b Beijing Key Laboratory for Theory and Technology of Advanced Battery Materials, College of Engineering, Peking University, Beijing 100871, China
E-mail: rzou@pku.edu.cn

Abstract

A stable Zn-based metal–organic framework has been synthesized and applied for CO₂ removal from syngas composed of CO and H₂ for the first time. Further study using the combination of Monte Carlo simulation and ideal adsorbed solution theory method demonstrates the CO₂ adsorption behavior and separation performance which have been further confirmed by breakthrough experiments.

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Article information

DOI: https://doi.org/10.1039/C5CE01320H
Article type: Communication
Submitted: 06 Jul 2015
Accepted: 03 Sep 2015
First published: 04 Sep 2015

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CrystEngComm, 2015,17, 8221-8225

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Experimental and theoretical investigation of a stable zinc-based metal–organic framework for CO₂ removal from syngas

R. Zhong, J. Liu, X. Huang, X. Yu, C. Sun, G. Chen and R. Zou, CrystEngComm, 2015, 17, 8221 DOI: 10.1039/C5CE01320H

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