Fabrication of Mn–CeOx/CNTs catalysts by a redox method and their performance in low-temperature NO reduction with NH3†
Abstract
Highly active Mn–CeOx/CNTs catalysts were first fabricated by a novel redox method, and a formation mechanism was proposed. The as-obtained catalyst possessed an amorphous structure, and high Ce3+/(Ce3+ + Ce4+) and Oα/(Oα + Oβ) ratios, which endowed it with 52.2–98.4% NO conversion at a weight hourly space velocity of 210 000 ml gcat−1 h−1.