Heterolytic cleavage of ammonia N–H bond by bifunctional activation in silica-grafted single site Ta(V)imido amido surface complex. Importance of the outer sphere NH3 assistance†
Abstract
* Corresponding authors
a
Université de Lyon, UMR 5265 « C2P2 », (UCBL Lyon 1- CPE Lyon -CNRS), École Supérieure Chimie Physique Electronique, 43 Boulevard du 11 Novembre 1918, BP 82077, Villeurbanne, France
E-mail:
e.p.goure@umail.leidenuniv.nl, priscilla.avenier@ifp.fr, jeanmarie.basset@kaust.edu.sa, quadrelli@cpe.fr
Fax: +33 (0)472431795
Tel: +33 (0)4724318 08
b
Departament de Quimica, Universitat Autònoma de Barcelona, 08193 Bellaterra, Spain
E-mail:
xavi@klingon.uab.es
Fax: +34 935812920
Tel: +34 935812173
c
Institut Charles Gerhardt, Université Montpellier 2, CNRS 5253, cc 1501, Place E. Bataillon, 34095 Montpellier, France
E-mail:
odile.eisenstein@univ-montp2.fr
Fax: +33 (0)467144839
Tel: +33 (0)467143306
E. Gouré, P. Avenier, X. Solans-Monfort, L. Veyre, A. Baudouin, Y. Kaya, M. Taoufik, J. Basset, O. Eisenstein and E. A. Quadrelli, New J. Chem., 2011, 35, 1011 DOI: 10.1039/C1NJ20032A
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