The first enantiocontrolled total synthesis of (–)-goniomitine, a new structural type of indole alkaloid of the Aspidosperma family isolated from the root bark of Gonioma malagasy, has been completed starting from a chiral cyclopentadienone synthon and establishes the absolute stereochemistry as 20R, 21S.
S. Takano, T. Sato, K. Inomata and K. Ogasawara, J. Chem. Soc., Chem. Commun., 1991, 462 DOI: 10.1039/C39910000462
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