The first asymmetric total synthesis of lycoposerramine-R, a Lycopodium alkaloid possessing a novel skeleton, was accomplished by a strategy featuring the stereoselective intramolecular aldol cyclization giving a cis-fused 5/6 bicyclic skeleton and a new method for the construction of the pyridone ring via the aza-Wittig reaction.
H. Ishida, S. Kimura, N. Kogure, M. Kitajima and H. Takayama, Org. Biomol. Chem., 2015, 13, 7762 DOI: 10.1039/C5OB00827A
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